Perovskite solar cells are promising candidates for next-generation photovoltaics. However, their performance as multi-scale devices is determined by complex interactions between their constituent layers. This creates a vast combinatorial space of possible materials and device architectures, making the conventional experimental-based screening process slow and expensive. Machine learning models try to address this problem, but they only focus on individual material properties or neglect the important geometric information of the perovskite crystal. To address this problem, we propose to predict perovskite solar cell power conversion efficiency with a geometric-aware co-attention (Solar-GECO) model. Solar-GECO combines a geometric graph neural network (GNN) - that directly encodes the atomic structure of the perovskite absorber - with language model embeddings that process the textual strings representing the chemical compounds of the transport layers and other device components. Solar-GECO also integrates a co-attention module to capture intra-layer dependencies and inter-layer interactions, while a probabilistic regression head predicts both power conversion efficiency (PCE) and its associated uncertainty. Solar-GECO achieves state-of-the-art performance, significantly outperforming several baselines, reducing the mean absolute error (MAE) for PCE prediction from 3.066 to 2.936 compared to semantic GNN (the previous state-of-the-art model). Solar-GECO demonstrates that integrating geometric and textual information provides a more powerful and accurate framework for PCE prediction.

Abstract-- We present Phaser, a flexible system that directs narrow-beam laser light to moving robots for concurrent wireless power delivery and communication. We design a semiautomatic calibration procedure to enable fusion of stereo-vision-based 3D robot tracking with high-power beam steering, and a low-power optical communication scheme that reuses the laser light as a data channel. We fabricate a Phaser prototype using off-the-shelf hardware and evaluate its performance with battery-free autonomous robots. We demonstrate Phaser fully powering gram-scale battery-free robots to nearly 2x higher speeds than prior work while simultaneously controlling them to navigate around obstacles and along paths. Code, an open-source design guide, and a demonstration video of Phaser is available at https: //mobilex.cs.columbia.edu/phaser/. Mobile, autonomous robots play an increasingly important role in today's world, with the potential to perform tasks in warehouses, factories, and homes and conduct advanced environmental explorations [1]. However, the significant power needed for locomotion, on-board computation, and communication presents a key barrier to the broader deployment of such robots. Given the energy density of current batteries [2], most autonomous robots today either remain tethered by charging wires or must routinely return to charging stations, reducing deployment time. This problem is exacerbated in miniaturized robots, which cannot support the 100s of milligrams of battery payload [3]-[7] needed for extended operation, even on their milliwatt power budgets.

Small racing quadcopters carrying explosives, known as first-person-view drones or FPVs, have become the dominant weapon in the war in Ukraine. Now, some are fitted with solar cells so they can wait for extended periods to ambush targets, turning them into a new type of land mine. "The drone can sit by a road or choke point and when it acquires its target, it can then do a quick sprint to the target," says Robert Bunker at US consultancy firm C/O Futures. Drone ambushes, where the devices land beside a road or on a building and wait for a target, are already commonly carried out by both Russian and Ukrainian forces. But even with their engines turned off, their camera and radio communications drain the drones' battery, limiting waiting time to a few hours at best.

We demonstrate a machine learning (ML) approach that accurately predicts the current-voltage behavior of 3D/2D-structured (FAMA)Pb(IBr)3/OABr hybrid organic-inorganic halide perovskite (HOIP) solar cells under AM1.5 illumination. Our neural network algorithm is trained on measured responses from several hundred HOIP solar cells, using three simple optical measurements of constituent HOIP films as input: optical transmission spectrum, spectrally-resolved photoluminescence, and time-resolved photoluminescence, from which we predict the open-circuit voltage (Voc), short-circuit current (Jsc), and fill factors (FF) values of solar cells that contain the HOIP active layers. Determined average prediction accuracies for 95 % of the predicted Voc, Jsc, and FF values are 91%, 94% and 89%, respectively, with R2 coefficients of determination of 0.47, 0.77, and 0.58, respectively. Quantifying the connection between ML predictions and physical parameters extracted from the measured HOIP films optical properties, allows us to identify the most significant parameters influencing the prediction results. With separate ML-classifying algorithms, we identify degraded solar cells using the same optical input data, achieving over 90% classification accuracy through support vector machine, cross entropy loss, and artificial neural network algorithms. To our knowledge, the demonstrated regression and classification work is the first to use ML to predict device photovoltaic properties solely from the optical properties of constituent materials.

We propose LightLLM, a model that fine tunes pre-trained large language models (LLMs) for light-based sensing tasks. It integrates a sensor data encoder to extract key features, a contextual prompt to provide environmental information, and a fusion layer to combine these inputs into a unified representation. This combined input is then processed by the pre-trained LLM, which remains frozen while being fine-tuned through the addition of lightweight, trainable components, allowing the model to adapt to new tasks without altering its original parameters. This approach enables flexible adaptation of LLM to specialized light sensing tasks with minimal computational overhead and retraining effort. We have implemented LightLLM for three light sensing tasks: light-based localization, outdoor solar forecasting, and indoor solar estimation. Using real-world experimental datasets, we demonstrate that LightLLM significantly outperforms state-of-the-art methods, achieving 4.4x improvement in localization accuracy and 3.4x improvement in indoor solar estimation when tested in previously unseen environments. We further demonstrate that LightLLM outperforms ChatGPT-4 with direct prompting, highlighting the advantages of LightLLM's specialized architecture for sensor data fusion with textual prompts.

We present a simulation of various active learning strategies for the discovery of polymer solar cell donor/acceptor pairs using data extracted from the literature spanning $\sim$20 years by a natural language processing pipeline. While data-driven methods have been well established to discover novel materials faster than Edisonian trial-and-error approaches, their benefits have not been quantified for material discovery problems that can take decades. Our approach demonstrates a potential reduction in discovery time by approximately 75 %, equivalent to a 15 year acceleration in material innovation. Our pipeline enables us to extract data from greater than 3300 papers which is $\sim$5 times larger and therefore more diverse than similar data sets reported by others. We also trained machine learning models to predict the power conversion efficiency and used our model to identify promising donor-acceptor combinations that are as yet unreported. We thus demonstrate a pipeline that goes from published literature to extracted material property data which in turn is used to obtain data-driven insights. Our insights include active learning strategies that can be used to train strong predictive models of material properties or be robust to the initial material system used. This work provides a valuable framework for data-driven research in materials science.

This work presents a set of optimal machine learning (ML) models to represent the temporal degradation suffered by the power conversion efficiency (PCE) of polymeric organic solar cells (OSCs) with a multilayer structure ITO/PEDOT:PSS/P3HT:PCBM/Al. To that aim, we generated a database with 996 entries, which includes up to 7 variables regarding both the manufacturing process and environmental conditions for more than 180 days. Then, we relied on a software framework that brings together a conglomeration of automated ML protocols that execute sequentially against our database by simply command-line interface. This easily permits hyper-optimizing and randomizing seeds of the ML models through exhaustive benchmarking so that optimal models are obtained. The accuracy achieved reaches values of the coefficient determination (R2) widely exceeding 0.90, whereas the root mean squared error (RMSE), sum of squared error (SSE), and mean absolute error (MAE)>1% of the target value, the PCE. Additionally, we contribute with validated models able to screen the behavior of OSCs never seen in the database. In that case, R2~0.96-0.97 and RMSE~1%, thus confirming the reliability of the proposal to predict. For comparative purposes, classical Bayesian regression fitting based on non-linear mean squares (LMS) are also presented, which only perform sufficiently for univariate cases of single OSCs. Hence they fail to outperform the breadth of the capabilities shown by the ML models. Finally, thanks to the standardized results offered by the ML framework, we study the dependencies between the variables of the dataset and their implications for the optimal performance and stability of the OSCs. Reproducibility is ensured by a standardized report altogether with the dataset, which are publicly available at Github.

Through the generation of a dataset of accurate band gaps for perovskite materials and the use of machine learning methods, several promising halide perovskites are identified for photovoltaic applications. As we integrate solar energy into our daily lives, it has become important to find materials that efficiently convert sunlight into electricity. While silicon has dominated solar technology so far, there is also a steady turn towards materials known as perovskites due to their lower costs and simpler manufacturing processes. The challenge, however, has been to find perovskites with the right "band gap": a specific energy range that determines how efficiently a material can absorb sunlight and convert it into electricity without losing it as heat. Now, an EPFL research project led by Haiyuan Wang and Alfredo Pasquarello, with collaborators in Shanghai and in Louvain-La-Neuve, have developed a method that combines advanced computational techniques with machine-learning to search for optimal perovskite materials for photovoltaic applications.